Electrolytic cell engineering and device optimization for electrosynthesis of e-biofuels via co-valo

来源 :化学科学与工程前沿 | 被引量 : 0次 | 上传用户:dt
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
Utilizing CO2 in an electro-chemical process and synthesizing value-added chemicals are amongst the few viable and scalable pathways in carbon capture and utilization technologies.CO2 electro-reduction is also counted as one of the main options entailing less fossil fuel consumption and as a future electrical energy storage strategy.The current study aims at developing a new electrochemical platform to produce low-carbon e-biofuel through multifunctional electrosynthesis and integrated covalorisation of biomass feedstocks with captured CO2.In this approach,CO2 is reduced at the cathode to produce drop-in fuels (e.g.,methanol) while value-added chemicals (e.g.,selective oxidation of alcohols,aldehydes,carboxylic acids and amines/amides) are produced at the anode.In this work,a numerical model of a continuous-flow design considering various anodic and cathodic reactions was built to determine the most techno-economically feasible configurations from the aspects of energy efficiency,environment impact and economical values.The reactor design was then optimized via parametric analysis.
其他文献